Three-dimensional nanoscale control of magnetism in crystalline Yttrium Iron Garnet
Authors: Valerio Levati, Matteo Vitali, Andrea Del Giacco, Nicola Pellizzi, Raffaele Silvani, Luca Ciaccarini Mavilla, Marco Madami, Irene Biancardi, Davide Girardi, Matteo Panzeri, Piero Florio, David Breitbach, Philipp Pirro, Ludovica Rovatti, Nora Lecis, Federico Maspero, Riccardo Bertacco, Giacomo Corrielli, Roberto Osellame, Valeria Russo, Andrea Li Bassi, Silvia Tacchi, Daniela Petti, Edoardo Albisetti
AI-generated Key Points
- Authors present a novel approach to nanostructuring crystalline Yttrium Iron Garnet (YIG) thin films using a focused UV laser
- Process enhances perpendicular magnetic anisotropy while maintaining material's crystalline quality
- Modulation of magnetic properties is highly confined at nanoscale in lateral and vertical directions, providing precise control over depth and extent of anisotropy profiles within the material's volume
- Collaborative effort involving various experimental and theoretical techniques such as static magnetic characterization, Brillouin Light Scattering (BLS) measurements, micromagnetic simulations, structural and optical characterization, Raman measurements, fabrication of spin-wave antennas, and finite element method (FEM) laser heating modeling
- Significant advancements demonstrated in spin-wave band structure tuning, spatial localization within the volume, and non-reciprocity
- Development paves the way for three-dimensional magnonic crystals with unique functionalities
- Research supported by European Union programs Horizon 2020 and Next Generation EU, Italian Ministry for University and Research grants, Fondazione Cariplo, Deutsche Forschungsgemeinschaft (DFG)
- Represents significant advancement in magnonics and magneto-optic devices through laser nanofabrication technique for creating three-dimensional magnetic systems based on crystalline YIG thin films
- Findings open up new possibilities for innovative functionalities in future technologies related to magnonics and nanomagnetism
Abstract: The exceptional magnetic, optical and phononic properties of Yttrium Iron Garnet (YIG) make it unique for spin-wave based and photonic applications. Yet, nanostructuring crystalline YIG and manipulating its magnetism in a non-destructive way is an outstanding challenge, and so far mostly limited to two-dimensional capabilities. Here, we show that irradiation of single-crystal YIG films with a focused UV laser drives a stable, giant enhancement of the perpendicular magnetic anisotropy, preserving the crystalline quality. This modulation is highly confined at the nanoscale in both the lateral and vertical directions, and its extension within the volume can be finely tuned with a continuous depth-control. By harnessing these three-dimensional anisotropy profiles, we demonstrate a large tuning of the spin-wave band structure, volume spatial localization, and non-reciprocity, realizing proof-of-principle 3D magnonic crystals. This straightforward, single-step, laser nanofabrication of three-dimensional magnetic systems based on crystalline YIG thin films opens the way to design novel functions in magnonic and magneto-optic devices.
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