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Abstract: This letter investigates the optimal allocation of large language model (LLM) inference workloads across heterogeneous edge data centers (DCs) over time. Each DC features on-site renewable generation and faces dynamic electricity prices and spatiotemporal variability in renewable availability. The central question is: how can inference workloads be optimally distributed to the DCs to minimize energy consumption, carbon emissions, and water usage while enhancing user experience? This letter proposes a novel optimization model for LLM service providers to reduce operational costs and environmental impacts. Numerical results validate the efficacy of the proposed approach.