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Pulse-Duration Control of Subcycle Multiband Electron Dynamics Extends the High-Harmonic Cutoff in a Light-Driven Insulator

Hortense Allegre, Simon V. B. Jensen, Joseph J. Broughton, Tim Klee, Yan Li, Jon P. Marangos, Nicolas Tancogne-Dejean, Angel Rubio, John W. G. Tisch, Mary R. Matthews

arXiv: 2608.06129v1 (physics.optics)

Résumé : We demonstrate pathway-selective control of extreme-ultraviolet high-harmonic generation by jointly tuning laser pulse duration ($5$ - $29$ fs) and intensity ($0.8$ - $74$ TW/cm$^2$). Many-cycle pulses at moderate intensities, $\sim 6$ TW/cm$^2$, promote cumulative carrier transfer over successive optical cycles, progressively accessing higher conduction bands. In contrast, few-cycle, high-intensity, $\sim 22$ TW/cm$^2$, pulses drive subcycle multiband dynamics that reach $25$ - $50$ eV photon energies before decoherence can suppress coherent emission. These results reveal pulse duration and intensity as decisive control knobs for high-harmonic emission, opening a route to band-structure-guided pulse design for higher energy extreme-ultraviolet light sources.

Soumis à arXiv le 06 Aoû. 2026